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Electrooxidative C–H Functionalization of Heteroarenes. Thiocyanation of Pyrazolo[1,5-a]pyrimidines

Kokorekin V. A., Yaubasarova R. R., Neverov S. V., Petrosyan V. A.
European Journal of Organic Chemistry
Vol.2019, Issue26, P. 4233-4238
Опубликовано: 2019
Тип ресурса: Статья

DOI:10.1002/ejoc.201900390

Аннотация:
Efficient electrooxidative C–H thiocyanation of both high and low reactive pyrazolo[1,5-a]pyrimidines using a new system of complementary approaches has been developed. Advantages of this promising strategy are the undivided cell, mild conditions, and readily available reagents as well as feasible scaling up process and transformation of the synthesized aryl thiocyanates to new thiols. Also, target thiocyanates were found to have pronounced antifungal activity. © 2019 WILEY-VCH Verlag GmbH & Co. KGaA, Weinheim
Ключевые слова:
Anodic C–H thiocyanation; C–S coupling; Potentiostatic electrolysis; Pyrazolo[1,5-a]pyrimidines; Thiocyanate ion
Язык текста: Английский
ISSN: 1099-0690
Kokorekin V. A. Vladimir Alekseevich 1987-
Yaubasarova R. R.
Neverov S. V.
Petrosyan V. A.
Кокорекин В. А. Владимир Алексеевич 1987-
Яубасарова Р. Р.
Неверов С. В.
Петросян В. А.
Electrooxidative C–H Functionalization of Heteroarenes. Thiocyanation of Pyrazolo[1,5-a]pyrimidines
Текст визуальный непосредственный
European Journal of Organic Chemistry
Wiley Interscience
Vol.2019, Issue26 P. 4233-4238
2019
Статья
Anodic C–H thiocyanation C–S coupling Potentiostatic electrolysis Pyrazolo[1,5-a]pyrimidines Thiocyanate ion
Efficient electrooxidative C–H thiocyanation of both high and low reactive pyrazolo[1,5-a]pyrimidines using a new system of complementary approaches has been developed. Advantages of this promising strategy are the undivided cell, mild conditions, and readily available reagents as well as feasible scaling up process and transformation of the synthesized aryl thiocyanates to new thiols. Also, target thiocyanates were found to have pronounced antifungal activity. © 2019 WILEY-VCH Verlag GmbH & Co. KGaA, Weinheim